Transition metal, non-metal carbonyl clustrs as supports for unusual acetylide reactivity
DSpace at IIT Bombay
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Title |
Transition metal, non-metal carbonyl clustrs as supports for unusual acetylide reactivity
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Creator |
MATHUR, P
BHUNIA, AK SRINIVASU, C MOBIN, SM |
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Subject |
acetylide
carbonyl chalcogen cluster mixed-metal |
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Description |
Group 16 elements serve as useful bridging and stabilising single atom ligands in mixed-metal carbonyl complexes and impart unusual reactivity on coordinated acetylenic moieties. Reactions of [Fe-3(CO)(9)(mu(3)-E)(2)](E = S, or Se) with mononuclearacetylide complexes, [CPM(CO)(3-x)(CCR)] (M = Mo or W, x = 0, R = Ph; M = Fe, x = 1, R = Ph or ferrocenyl) under facile conditions yield complexes featuring acetylide coupling, acetylide-flip and formation of oxo and acetylide-bridged complexes. In presence of free acetylenes, unusual ligand systems arising from C-S bond formation are observed and under certain conditions, formation of quinones by coupling of acetylenes with carbon monoxide is facilitated.
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Publisher |
TAYLOR & FRANCIS LTD
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Date |
2011-10-22T19:15:01Z
2011-12-15T09:10:46Z 2011-10-22T19:15:01Z 2011-12-15T09:10:46Z 2004 |
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Type |
Article; Proceedings Paper
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Identifier |
PHOSPHORUS SULFUR AND SILICON AND THE RELATED ELEMENTS,179,899-901
1042-6507 http://dx.doi.org/10.1080/10426500490428861 http://dspace.library.iitb.ac.in/xmlui/handle/10054/14968 http://hdl.handle.net/100/1647 |
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Source |
10th International Symposium on Inorganic Ring Systems (IRIS 10),Burlington, VT,AUG 17-22, 2003
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Language |
English
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