Molecular complexity from aromatics - An efficient route to 1,8-dimethyl-5-spirocyclopropanetricyclo[6.3.0.0(2,6)]undec-10-one: A potential intermediate for synthesis of ceratopicanol
DSpace at IIT Bombay
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Title |
Molecular complexity from aromatics - An efficient route to 1,8-dimethyl-5-spirocyclopropanetricyclo[6.3.0.0(2,6)]undec-10-one: A potential intermediate for synthesis of ceratopicanol
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Creator |
SINGH, V
CHANDRA, G MOBIN, SM |
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Subject |
1st total-synthesis
linear triquinane cyclization reactions holosynthon concept acid (+/-)-ceratopicanol sesquiterpenoids (+/-)-hirsutene rearrangement hypnophilin cycloaddition oxa-di-pi-methane rearrangement triquinanes diels-alder reaction |
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Description |
A new stereoselective synthesis of linearly fused triquinane intermediate from a simple aromatic precursor is described. Cycloaddition of cycloliexa-2.4-dienone and photochemical oxa-di-pi-methane rearrangement in a functionalized tricycloundecenone are the key features of our methodology.
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Publisher |
GEORG THIEME VERLAG KG
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Date |
2011-07-30T08:36:08Z
2011-12-26T12:52:45Z 2011-12-27T05:39:37Z 2011-07-30T08:36:08Z 2011-12-26T12:52:45Z 2011-12-27T05:39:37Z 2008 |
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Type |
Article
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Identifier |
SYNLETT, (15), 2267-2270
0936-5214 http://dx.doi.org/10.1055/s-2008-1078592 http://dspace.library.iitb.ac.in/xmlui/handle/10054/7904 http://hdl.handle.net/10054/7904 |
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Language |
en
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