Synthesis of some functionalised isomeric bis(ethylenedithio)tetrathiafulvalene (BEDT-TTF) and dithiophenetetrathiafulvalene (DTTTF) pi-donors
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Title |
Synthesis of some functionalised isomeric bis(ethylenedithio)tetrathiafulvalene (BEDT-TTF) and dithiophenetetrathiafulvalene (DTTTF) pi-donors
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Creator |
KUMAR, EVKS
SINGH, JD SINGH, HB DAS, K VERGHESE, B |
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Subject |
electron-donors
crystal-structure tetrathiafulvalene derivatives organic metals spacer groups systems dithiaheterocycles chemistry analog anion |
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Description |
The synthesis of some functionalised isomeric, symmetrical tetrathiafulvalene derivatives containing 4,5-(ethylenedithio)-1,3-dithiole and 4,5-(propylenedithio)-1,3-dithiole units is described. These contain hydroxy, chloro and cyano functionalities (4, 6, 9 and 12). Interestingly, attempted coupling of 4,5-bis(propargylthio)-1,3-dithiole-2-thione 13, to obtain the corresponding TTF, 14 afforded the novel thione, 5-methylthieno[2,3-d]-1,3-dithiole-2-thione 15. Self coupling of thione 15 in the presence of trimethyl phosphite afforded new functionalised dithiophenetetrathiafulvalene 16. The X-ray crysal structures of 4,5-bis(propargyldithio)-1,3-dithiole-2-thione 13 and 5-methylthieno[2,3-d]-1,3-dithiole-2-thione 15 are described. (C) 1997 .
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Publisher |
PERGAMON-ELSEVIER SCIENCE LTD
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Date |
2011-08-26T22:15:42Z
2011-12-26T12:57:36Z 2011-12-27T05:44:11Z 2011-08-26T22:15:42Z 2011-12-26T12:57:36Z 2011-12-27T05:44:11Z 1997 |
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Type |
Article
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Identifier |
TETRAHEDRON, 53(34), 11627-11644
0040-4020 http://dspace.library.iitb.ac.in/xmlui/handle/10054/11450 http://hdl.handle.net/10054/11450 |
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Language |
en
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