Synthesis of dithiaporphyrin-based singlet-singlet energy transfer systems
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Title |
Synthesis of dithiaporphyrin-based singlet-singlet energy transfer systems
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Creator |
KUMARESAN, D
AGARWAL, N RAVIKANTH, M |
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Subject |
unsymmetrical porphyrin dimers
electrochemical properties coupling reactions arrays design 21-thiaporphyrin nickel(ii) oligomers dynamics spectra |
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Description |
The synthesis of the first alkynyl core-modified porphyrin building block, 5,10,15,20-tetrakis(4-ethynylphenyl)-21,23-dithiaporphyrin (N2S2 core), is reported. The building block was used to construct donor-appended dithiaporphyrin systems under mild palladium-coupling conditions. The porphyrin building block appended to four boron-dipyrrin units, (BDPY)(4)S2TPP, did not show any energy transfer from the BDPY unit to the central dithiaporphyrin core. However, the pentaporphyrin containing a central dithiaporphyrin sub-unit and four peripheral normal porphyrin sub-units (N-4 core) showed efficient energy transfer from the peripheral N-4 porphyrins to the central N2S2 porphyrin.
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Publisher |
ROYAL SOC CHEMISTRY
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Date |
2011-08-28T21:00:34Z
2011-12-26T12:58:12Z 2011-12-27T05:47:45Z 2011-08-28T21:00:34Z 2011-12-26T12:58:12Z 2011-12-27T05:47:45Z 2001 |
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Type |
Article
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Identifier |
JOURNAL OF THE CHEMICAL SOCIETY-PERKIN TRANSACTIONS 1, (14), 1644-1648
1472-7781 http://dx.doi.org/10.1039/b102349g http://dspace.library.iitb.ac.in/xmlui/handle/10054/11843 http://hdl.handle.net/10054/11843 |
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Language |
en
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