Interaction of 3-hydroxybenzoate-6-hydroxylase with cibacron blue
DSpace at IIT Bombay
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Title |
Interaction of 3-hydroxybenzoate-6-hydroxylase with cibacron blue
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Creator |
SUMATHI, S
DASGUPTA, D |
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Subject |
dinucleotide fold
sepharose chromatography lactate-dehydrogenase klebsiella-pneumoniae glutamine-synthetase dextran-sepharose purification proteins binding 6-hydroxylase cibacron blue circular dichroism competitive flavin fluorescence 3-hydroxybenzoate inhibition uncompetitive monooxygenase 3-hydroxybenzoate-6-hydroxylase |
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Description |
Cibacron blue is a potent inhibitor of 3-HBA-6-hydroxylase at a concentration < 1 mu M. Kinetic analyses revealed that at a concentration below 0.5 mu M the dye behaves as an uncompetitive inhibitor with respect to 3-HBA and competes with NADH for the same site on the enzyme. The alteration of the near-UV CD spectrum and quenching of the emission fluorescence of the enzyme by cibacron blue indicates a significant alteration in the environment of aromatic amino acid residues due to a stacking interaction and subtle conformatiodnal changes in the enzyme. The concentration-dependent quenching of the intrinsic fluorescence of the enzyme by cibacron blue was employed to determine the binding parameters such as association constant (K-a) and stoichiometry (r) for the enzyme-dye complex.
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Publisher |
TAYLOR & FRANCIS LTD
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Date |
2011-08-31T00:51:24Z
2011-12-26T12:59:15Z 2011-12-27T05:50:21Z 2011-08-31T00:51:24Z 2011-12-26T12:59:15Z 2011-12-27T05:50:21Z 2006 |
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Type |
Article
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Identifier |
JOURNAL OF ENZYME INHIBITION AND MEDICINAL CHEMISTRY, 21(1), 47-53
1475-6366 http://dx.doi.org/10.1080/02781070500323047 http://dspace.library.iitb.ac.in/xmlui/handle/10054/12523 http://hdl.handle.net/10054/12523 |
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Language |
en
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