Effect of achiral and mixed chiral ligands on the asymmetric synthesis of γ-nitrophosphonates via Michael addition
DSpace at IIT Bombay
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Title |
Effect of achiral and mixed chiral ligands on the asymmetric synthesis of γ-nitrophosphonates via Michael addition
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Creator |
RAI, VISHAL
NAMBOOTHIRI, IRISHI NN |
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Subject |
enantioselectivity
stereoselectivity catalysts |
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Description |
Change in the diastereo- and/or enantioselectivity were observed when the Li–cinchonine catalyzed conjugate addition of phosphonates to nitroalkenes was carried out in the presence of achiral/chiral additives. Although the conjugate addition in the absence of such additives proceeded in better yields and selectivities as reported previously, the dramatic change in selectivity in the presence of additives provides an opportunity to synthesize different stereoisomers of the product, γ-nitrophosphonate, using primarily the same chiral source.
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Publisher |
Elsevier
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Date |
2009-02-16T12:00:20Z
2011-11-25T17:00:55Z 2011-12-26T13:05:59Z 2011-12-27T05:51:52Z 2009-02-16T12:00:20Z 2011-11-25T17:00:55Z 2011-12-26T13:05:59Z 2011-12-27T05:51:52Z 2008 |
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Type |
Article
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Identifier |
Tetrahedron: Asymmetry 19(7), 1-8
0957-4166 http://dx.doi.org/10.1016/j.tetasy.2008.03.006 http://hdl.handle.net/10054/661 http://dspace.library.iitb.ac.in/xmlui/handle/10054/661 |
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Language |
en
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