Stereoselective Synthesis of Trifluoromethyl Analogues of Polyhydroxypyrrolidines
DSpace at IIT Bombay
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Title |
Stereoselective Synthesis of Trifluoromethyl Analogues of Polyhydroxypyrrolidines
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Creator |
KHANGAROT, RK
KALIAPPAN, KP |
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Subject |
Synthetic methods
Nitrogen heterocycles Fluorine Nucleophilic addition Diastereoselectivity FLUORINATED AMINO-ACIDS COPE-HOUSE CYCLIZATION NITRONES EN-ROUTE CYCLIC NITRONES NUCLEOPHILIC TRIFLUOROMETHYLATION THERAPEUTIC APPLICATIONS RADICAMINE-B POLYHYDROXYLATED PYRROLIDINES ANGYLOCALYX-BOUTIQUEANUS GLYCOSIDASE INHIBITORS |
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Description |
Incorporation of fluorine atoms into organic molecules significantly enhances many of their properties, such as solubility, metabolic stability, and bioavailability. Among organofluorine molecules, trifluoromethylated compounds play a unique and important role in agricultural and medicinal chemistry. An efficient strategy for the synthesis of a variety of trifluoromethylated polyhydroxypyrrolidines is described. This strategy involves a diastereoselective nucleophilic addition reaciton of trimethyl(trifluoromethyl)silane to sugar-derived cyclic nitrones followed by reductive NO bond cleavage and removal of benzyl groups.
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Publisher |
WILEY-V C H VERLAG GMBH
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Date |
2014-10-16T06:35:39Z
2014-10-16T06:35:39Z 2013 |
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Type |
Article
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Identifier |
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY, (13)2692-2698
http://dx.doi.org/10.1002/ejoc.201201599 http://dspace.library.iitb.ac.in/jspui/handle/100/15448 |
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Language |
en
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