Diastereo- and enantioselective synthesis of densely functionalized cyclohexanones via double Michael addition of curcumins with nitroalkenes
DSpace at IIT Bombay
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Title |
Diastereo- and enantioselective synthesis of densely functionalized cyclohexanones via double Michael addition of curcumins with nitroalkenes
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Creator |
AYYAGARI, N
NAMBOOTHIRI, INN |
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Subject |
BIFUNCTIONAL THIOUREA
CASCADE REACTIONS STEREOSELECTIVE-SYNTHESIS ASYMMETRIC CATALYSIS EFFICIENT SYNTHESIS CONJUGATE ADDITION DOMINO REACTIONS ANALOGS DERIVATIVES ORGANOCATALYSTS |
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Description |
The asymmetric double Michael additions of curcumins to nitroalkenes to afford highly functionalized cyclohexanones have been carried out for the first time. A combination of a dihydrocinchonine-thiourea organocatalyst and K2CO3 was found to be the most effective in obtaining the desired cyclohexanones in good yield, diastereoselectivity and enantioselectivity. (C) 2012 Elsevier Ltd. All rights reserved.
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Publisher |
PERGAMON-ELSEVIER SCIENCE LTD
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Date |
2014-10-17T05:28:50Z
2014-10-17T05:28:50Z 2012 |
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Type |
Article
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Identifier |
TETRAHEDRON-ASYMMETRY, 23(8)605-610
http://dx.doi.org/10.1016/j.tetasy.2012.04.011 http://dspace.library.iitb.ac.in/jspui/handle/100/16068 |
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Language |
en
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