Synthesis, spectral and structural studies of water soluble arene ruthenium (II) complexes containing 2,2′-dipyridyl-N-alkylimine ligand
DRS at CSIR-National Institute of Oceanography
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Title |
Synthesis, spectral and structural studies of water soluble arene ruthenium (II) complexes containing 2,2′-dipyridyl-N-alkylimine ligand
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Creator |
Singh, K.S.
Kaminsky, W. |
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Subject |
water soluble complexes
Ruthenium Dimethylpyridyl ketone Crystal structure |
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Description |
A series of water soluble complexes of general formula [(Eta sup(6)-arene) Ru ((C sub(5) H sub(4) N) sub(2) CNRi) Cl) PF sub(6) have been prepared by the reaction of [[(Eta sup(6)- arene) RuCl sub(2)) sub(2)) with appropriate 2,2’-dipyridyl-N-alkylimine ligands (dpNRi) in the presence of NH sub(4) PF sub(6) (where; R = Me or Et; arene = p-cymene, C sub(6) Me sub(6), C sub(6) H sub(6)). The 2,2’-dipyridyl-N-alkylimine ligands are prepared by reaction of 2,2’-dipyridyl ketone with the corresponding alkylamine. The complexes are readily obtained as air stable yellow to dark brown solids by simple stirring at room temperature. The complexes are isolated as their hexafluorophosphate salts and characterized on the basis of spectroscopic data. The molecular structure of representative complex ((Eta sup(6)-Csub(6) Me sub(6)) Ru ((C sub(5) H sub(4) N) sub(2) C= N-Me) Cl) PF sub(6) has been determined by single crystal X-ray diffraction studies.
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Date |
2011-01-04T07:01:11Z
2011-01-04T07:01:11Z 2011 |
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Type |
Journal Article
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Identifier |
Inorganica Chimica Acta, vol.365(1); 2011; 487-491
http://drs.nio.org/drs/handle/2264/3768 |
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Language |
en
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Rights |
An edited version of this paper was published by Elsevier. Copyright [2011] Elsevier
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Publisher |
Elsevier
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