ICB3E Induces INOS Expression by ROS-Dependent JNK and ERK Activation for Apoptosis of Leukemic Cells
EPrints@IICB
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Title |
ICB3E Induces INOS Expression by ROS-Dependent JNK and ERK Activation for Apoptosis of Leukemic Cells |
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Creator |
Biswas, Nabendu
Mahato, Sanjit Kumar Acharya Chowdhury, Avik haudhuri, Jaydeep C Manna, Anirban Vinayagam, Jayaraman Chatterjee, Sourav Jaisankar , P Chaudhuri, Utpal Bandyopadhyay, Santu |
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Subject |
Cancer Biology and Inflammatory Disorder Division
Chemistry |
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Description |
The role of c-Jun N terminal Kinase (JNK) has been well documented in various cellular stresses where it leads to cell death. Similarly, extracellular signal-regulated kinase (ERK) which was identified as a signalling molecule for survival pathway has been shown recently to be involved in apoptosis also. Recently we reported that ICB3E, a synthetic analogue of Piper betle leaf-derived apoptosis-inducing agent hydroxychavicol (HCH), possesses anti-chronic myeloid leukemia (CML) acitivity in vitro and in vivo without insight on mechanism of action. Here we report that ICB3E is three to four times more potent than HCH in inducing apoptosis of leukemic cells without having appreciable effects on normal human peripheral blood mononuclear cells, mouse fibroblast cell line NIH3T3 and monkey kidney epithelial cell line Vero. ICB3E causes early accumulation of mitochondria-derived reactive oxygen species (ROS) in K562 cells. Unlike HCH, ICB3E treatment caused ROS dependent activation of both JNK, ERK and induced the expression of iNOS leading to generation of nitric oxide (NO). This causes cleavage of caspase 9, 3 and PARP leading to apoptosis. Lack of cleavage of caspase 8 and inability of blocking chimera antibody to DR5 or neutralizing antibody to Fas to reverse ICB3E-mediated apoptosis suggest the involvement of only intrinsic pathway. Our data reveal a novel ROS-dependent JNK/ERK-mediated iNOS activation pathway which leads to NO mediated cell death by ICB3E |
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Publisher |
Kluwer
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Date |
2012
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Type |
Article
PeerReviewed |
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Format |
application/pdf
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Identifier |
http://www.eprints.iicb.res.in/1481/1/APOPTOSIS___17(_6)__612%2D626;2012[6].pdf
Biswas, Nabendu and Mahato, Sanjit Kumar and Acharya Chowdhury, Avik and haudhuri, Jaydeep C and Manna, Anirban and Vinayagam, Jayaraman and Chatterjee, Sourav and Jaisankar , P and Chaudhuri, Utpal and Bandyopadhyay, Santu (2012) ICB3E Induces INOS Expression by ROS-Dependent JNK and ERK Activation for Apoptosis of Leukemic Cells. Apoptosis, 17 (6). pp. 612-626. |
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Relation |
http://dx.doi.org/10.1007/s10495-011-0695-9
http://www.eprints.iicb.res.in/1481/ |
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