<p class="BATitle">Template-free synthesis of hierarchical mesoporous carbon: Based on functional coal tar pitches with carboxylation and diketone structures</p>
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Title Statement |
<p class="BATitle">Template-free synthesis of hierarchical mesoporous carbon: Based on functional coal tar pitches with carboxylation and diketone structures</p> |
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Added Entry - Uncontrolled Name |
Wang, Haiyang ; The State Key Laboratory of Fine Chemicals, Dalian University of Technology, Dalian 116023, China
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Sinosteel Anshan Research Institute of Thermo-Energy Company Limited, Anshan 114044, China Zhu, Hongzhe ; Sinosteel Anshan Research Institute of Thermo-Energy Company Limited, Anshan 114044, China Qi, Debang ; The State Key Laboratory of Fine Chemicals, Dalian University of Technology, Dalian 116023, China Wang, Shoukai ; Sinosteel Anshan Research Institute of Thermo-Energy Company Limited, Anshan 114044, China Shen, Kaihua ; The State Key Laboratory of Fine Chemicals, Dalian University of Technology, Dalian 116023, China |
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Uncontrolled Index Term |
Carboxylation; Coal tar pitches; Electrochemical properties; Hierarchical porous carbons |
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Summary, etc. |
<p style="text-align: justify;">An efficient and easy template-free method for the preparation of hierarchical porous carbons (HPCs) has been developed using low-priced coal tar pitch (CP) as the starting material. Application of the diketone (-COCO-) radical provides a carbonyl methylene group for polycyclic aromatic hydrocarbons by condensation and produces an effective micro-mesoporous network with a high specific surface area. With the help of controlled Friedel-Crafts reaction and oxidation, carboxyl-functionalized CP is obtained as the stratified porous CP precursor, and the high-temperature decarboxylation (>230°C) helped in generating well-developed micro-mesoporous carbon. The total pore volume of porous carbon of 1277.3 and 1.45 cm<sup>3</sup>g<sup>-1</sup> the maximum BET surface area suggests that the rapid electrolyte ion exchange and charge transportability would be better for the electrochemical capacitor.</p> |
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Publication, Distribution, Etc. |
Indian Journal of Chemistry -Section A (IJCA) 2020-10-06 15:05:21 |
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Electronic Location and Access |
application/pdf http://op.niscair.res.in/index.php/IJCA/article/view/41279 |
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Data Source Entry |
Indian Journal of Chemistry -Section A (IJCA); ##issue.vol## 59, ##issue.no## 9 (2020): INDIAN JOURNAL OF CHEMISTRY - SECTION A |
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Language Note |
en |
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