Pyrene appended terpyridine derivatives as electrochemiluminescence material for OLEDs: Characterization of photo-physical, thermal and electrochemical properties
NOPR - NISCAIR Online Periodicals Repository
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Title |
Pyrene appended terpyridine derivatives as electrochemiluminescence material for OLEDs: Characterization of photo-physical, thermal and electrochemical properties
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Creator |
Umasankar, Gorakala
Busireddy, Manohar Reddy Kotamarthi, Bhanuprakash Karunakar, Galla V Rao, Vaidya Jayathirtha |
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Subject |
Terpyridine-pyrene derivatives
Fluorescence quantum yield Delayed fluorescence Phosphorescence Thermal stability Oxidation and reduction potentials OLED materials |
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Description |
1564-1574
Three new terpyridine appended pyrene derivatives (Pyr-Tp, Pyr-Ph-Tp, and Pyr-Bp-Tp) have been synthesized by condensation and Suzuki-Miyaura reaction. The photo-physical, electro-chemical and thermal properties of these compounds have been investigated in detail. DFT studies have been carried out to understand the structure-property relationships at the molecular level. Synthesized fluorophores displayed high quantum yield (70-96%) of fluorescence due to triplet to singlet intramolecular energy transfer, delayed fluorescence and positive solvatochromism indicating the presence of intra-molecular charge transfer excited state. In addition, they have high thermal decomposition temperature (Td: 390-450°C), melting temperature (Tm: 180-220°C) and further with suitable oxidation and reduction potentials makes them favourable molecules for OLED fabrications. |
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Date |
2020-10-13T06:09:50Z
2020-10-13T06:09:50Z 2020-10 |
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Type |
Article
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Identifier |
0975-0983(Online); 0376-4699(Print)
http://nopr.niscair.res.in/handle/123456789/55464 |
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Language |
en_US
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Rights |
CC Attribution-Noncommercial-No Derivative Works 2.5 India
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Publisher |
NISCAIR-CSIR, India
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Source |
IJC-B Vol.59B(10) [October 2020]
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