<p>Structural characterization of <em>catena</em>-[bis(μ-4-nitrobenzoato)-diaqua-calcium 4,4'-bipyridine] and <em>catena</em>-[bis(μ-4-nitrobenzoato)-diaqua-calcium 1H-1,2,4-triazole]</p>
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Title Statement |
<p>Structural characterization of <em>catena</em>-[bis(μ-4-nitrobenzoato)-diaqua-calcium 4,4'-bipyridine] and <em>catena</em>-[bis(μ-4-nitrobenzoato)-diaqua-calcium 1H-1,2,4-triazole]</p> |
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Added Entry - Uncontrolled Name |
Srinivasan, Bikshandarkoil R; GOA UNIVERSITY |
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Uncontrolled Index Term |
Synthetic and structural inorganic chemistry Calcium; 4-nitrobenzoate; 1,2,4-triazole; 4,4′-bipyridine; coordination polymer; edge-sharing {CaO8} polyhedra |
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Summary, etc. |
An attempted incorporation of N-donor ligand in the coordination sphere of Ca in the molecular solid [Ca(H<sub>2</sub>O)<sub>4</sub>(4-nba)<sub>2</sub>] (4-nba=4-nitrobenzoate) resulted in the formation of the one-dimensional (1D) coordination polymers <em>catena</em>-[bis(μ-4-nitrobenzoato)-diaqua-calcium 4,4'-bipyridine] <strong>1</strong> and <em>catena</em>-[bis(μ-4-nitrobenzoato)-diaqua-calcium 1H-1,2,4-triazole] <strong>2</strong> with the N-heterocycle functioning as a solvate. The syntheses, crystal structures and properties of [Ca(H<sub>2</sub>O)<sub>2</sub>(4-nba)<sub>2</sub>]·L (L=4,4′-bipyridine <strong>1</strong>; L=1H-1,2,4-triazole <strong>2</strong>) are reported. The central Ca(II) in <strong>1</strong> and <strong>2</strong> exhibits eight-coordination and the aqua ligands are terminal, while 4-nitrobenzoate functions as a μ<sub>2</sub>-bridging ligand. The μ<sub>2</sub>-η<sup>2</sup>:η<sup>1 </sup>tridentate binding mode of the 4-nba ligand results in the formation of an infinite chain of edge-sharing {CaO<sub>8</sub>} polyhedra flanked by the 4-nitrobenzoates. The solvate 4,4′-bipyridine in <strong>1</strong> (or 1,2,4-triazole in <strong>2</strong>) links adjacent polymeric chains with the aid of O-H∙∙∙N hydrogen bonding interactions. A comparative study of {CaO<sub>x</sub>} polyhedral linking in structurally characterized calcium coordination polymers based on 4-nitrobenzoate is described. |
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Publication, Distribution, Etc. |
Indian Journal of Chemistry -Section A (IJCA) 2021-09-22 10:23:28 |
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Electronic Location and Access |
application/pdf http://op.niscair.res.in/index.php/IJCA/article/view/45373 |
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Data Source Entry |
Indian Journal of Chemistry -Section A (IJCA); ##issue.vol## 60, ##issue.no## 6 (2021): INDIAN JOURNAL OF CHEMISTRY- SECTION A |
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Language Note |
en |
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Nonspecific Relationship Entry |
http://op.niscair.res.in/index.php/IJCA/article/download/45373/465545264 http://op.niscair.res.in/index.php/IJCA/article/download/45373/465545265 http://op.niscair.res.in/index.php/IJCA/article/download/45373/465545362 http://op.niscair.res.in/index.php/IJCA/article/download/45373/0 http://op.niscair.res.in/index.php/IJCA/article/download/45373/465545365 http://op.niscair.res.in/index.php/IJCA/article/download/45373/465545419 |
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